The SEGA consoles should look ok with H Samplerate 427 and Sampling phase somewhere around 270. The PS1 is very finicky for it because it has a habit of switching resolutions.
EDIT: Also, some Mega Drive/Genesis titles use 320×240 while some need 256×240.
EDIT 2: If H Samplerate 427 doesn’t look good even when you tweak the sampling phase, try 428 and then play with the sampling phase again.
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